Chemical Communications 2015-Jun
Tuning the cavities of zirconium-based MIL-140 frameworks to modulate CO2 adsorption.
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A combined experimental and computational study has revealed the interplay between the framework pore size and functionality on the CO2 adsorption performance of zirconium-based MIL-140 frameworks. The CO2-sorbent interactions were markedly influenced by pore-confinement effects which arise from the π-stacked arrangement of the ligands within the framework backbone.
